Synonyms for Discontent (same or very similar meaning)
WordNet sense 1 (a longing for something better than the present situation):
discontentment, discontentedness
WordNet sense 2 (in a state of sulky dissatisfaction):
dissatisfied
WordNet sense 3 (discontented as toward authority):
malcontent
WordNet sense 4 (showing or experiencing dissatisfaction or restless longing):
discontented
From the ODE community, based on WordNet
add/edit