Verb (used with object) : The love letter was calligraphed in a delicate hand.    From Dictionary.com. 

A photographic calligraph, whose letters were so fine as to require a microscope to see them, was placed at a distance of three hundred feet.    From Wordnik.com.  [Scientific American Supplement, No. 288, July 9, 1881] Reference

East Asia Culture booths will feature calligraph, opera mask, traditional pops and entertainment--a drumming group from LA, celestial dances and music.    From Wordnik.com.  [RELIGION Blog | dallasnews.com] Reference

Then again, I'm not one to hand calligraph a hundred invitations to an event when I can just lay it out as a pdf and have it printed.    From Wordnik.com.  [Original Signal - Transmitting Digg] Reference